Thermoelectricity evidence for quantum criticality in clean infinite-layer nickelate films

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20m

Description

Quantum criticality has become a central paradigm for understanding unconventional superconductivity. However, its manifestation in the newly discovered family of nickelates remains largely unexplored. In this work, we investigate the thermopower-to-temperature ratio ($S/T$) in parent NdNiO$_{2}$ (NNO) and Sm$_{0.95-x}$Ca$_{0.05}$Eu$_{x}$NiO$_{2}$ (SCE$_{x}$) films. In clean NNO samples, the opposite signs of $S/T$ and Hall coefficient ($R_{H}$) indicate that thermopower are dominated by quantum criticality rather than band theory. In SCE$_{x}$, a log$T$ dependence emerges once superconductivity is suppressed by a magnetic field, but deviates from this behavior at $T_{s}$. The positive correlation between $T_{s}$ and $T_{c}$ highlights the role of quantum critical behavior in nickelate superconductors. These findings emphasize the importance of quantum critical behavior in proximity to QCP in infinite-layer nickelates and further suggest a convergence of such behavior across different unconventional superconducting families.

Primary authors

Dr Chihao Li (State Key Laboratory of Surface Physics, Department of Physics, Fudan University, Shanghai 200438, China) Prof. Danfeng Li (Department of Physics, City University of Hong Kong, Kowloon, Hong Kong SAR, China) Prof. Donglai Feng (New Cornerstone Science Laboratory, Hefei National Laboratory, Hefei 230088, China) Prof. Haichao Xu (State Key Laboratory of Surface Physics, Department of Physics, Fudan University, Shanghai 200438, China) Prof. Liang Qiao (School of Physics, University of Electronic Science and Technology of China, Chengdu, China) Dr Mingwei Yang (Department of Physics, City University of Hong Kong, Kowloon, Hong Kong SAR, China) Prof. Rui Peng (State Key Laboratory of Surface Physics, Department of Physics, Fudan University, Shanghai 200438, China) Prof. Shiyan Li (State Key Laboratory of Surface Physics, Department of Physics, Fudan University, Shanghai 200438, China) Dr Xu Zhang (State Key Laboratory of Surface Physics, Department of Physics, Fudan University, Shanghai 200438, China) Dr Yan Zhao (School of Physics, University of Electronic Science and Technology of China, Chengdu, China) Dr Zhitong An (State Key Laboratory of Surface Physics, Department of Physics, Fudan University, Shanghai 200438, China)

Presentation materials